Skeletal Structure
Skeletal Structure mxw142So now we know that monomers can be ‘strung’ together to form a long molecule called a polymer. Perhaps you are imaging that it looks like a tiny piece of string or spaghetti – and in many cases, we can simplify the drawing of the polymer by just drawing the skeletal structure as a squiggly line. In such drawings of skeletal structures, like those shown in Figure 1.9, we don’t draw out the specific chemical structure, but the lines are supposed to represent the polymer backbone and can help us visualize higher order structure. Because a polymer doesn’t just have to be a linear – it can be much more complicated than that. It can be branched – like a tree – or it can be network, where all the strings are connected to each other at linking points called crosslinks. The skeletal structure of a polymer significantly affects its properties. For example, network polymers tend to hold their 3D shape much better than linear polymers; can you imagine trying to build a sculpture out of spaghetti?

Introduction to Polymers, Third Edition, CRC Press, 2011.
In addition to classifying polymers by their chemical structure, we also classify them based on their physical properties (Figure 1.3 in the text). There are three main types: thermoplastics, elastomers, and thermosets. Elastomers are stretchy – think “elastic”, like a rubber band. They can be stretched and deformed and return to their original shape because their 3D structure is held together by crosslinks (i.e. most elastomers are network polymers). Their unique properties are a function of their 3D network structure. Things like crosslink density affect their macroscale material properties. Thermosets are rigid that usually have a very high degree of crosslinking. When they are heated, they don’t often flow or soften, they usually just degrade (i.e., the bonds in the polymer are broken). This is in contrast to thermoplastics or thermosoftening polymers, which do flow upon heating. Thermoplastics are typically linear or branched and do not have that network structure to hold their shape (hence they flow when heated). Most commercial polymers are thermoplastics. They can be crystalline, semi-crystalline, or amorphous. Crystalline phases have a melting temperature (Tm). Amorphous phases can’t really “melt” because they are already amorphous (it’s not considered a phase transition), so we use the term glass transition temperature (Tg) to characterize their softening point. Tg might be a range of temperature over which the transition occurs.
Some polymers have characteristics of more than one of these classes. In a sense, it’s a continuum. For example, some elastomers can also be characterized either as a thermoplastic or thermoset.
PROBLEM 1
If a polymer becomes more flexible, then how do you think Tg will change?
- Increase
- Decrease
- Stay the same
ANSWER
B. Decrease
PROBLEM 2
If intermolecular interactions between polymers increase, then how will Tg change?
- Increase
- Decrease
- Stay the same
ANSWER 2
A. Increase